Arthur Simpson-Kent was detained by the authorities earlier, two days after the Ghanaian police became involved in the hunt for him.
The bodies of Sian Blake, 43, Zachary, eight, and Amon, four, were found in the garden of their London home on Tuesday.
The family had been reported missing on 16 December.
The Met Police said it had been "made aware of an arrest in Ghana" and was "working alongside the Ghanaian authorities but is not in a position to discuss further at this time".
Ms Blake and the couple's sons had not been not seen since 13 December and a missing persons inquiry launched on 16 December, after the NSPCC had raised concerns about their welfare.
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